Monolith free-standing plasmonic PAN/Ag/AgX(X = Br, I)nanofiber mat as easily recoverable visible-light-driven photocatalyst

Monolith free-standing plasmonic PAN/Ag/AgX(X = Br, I)nanofiber mat as easily recoverable visible-light-driven photocatalyst

论文摘要

Most efficient visible-light-responsive photocatalysts are in the form of powder, leading to the tedious separation from the reaction media. Herein, we developed a versatile method for the general synthesis of free-standing polyacrylonitrile(PAN)/Ag/AgX(X = Br, I) nanofiber mats, where fibrous PAN/Ag precursor was firstly prepared via an electroless plating strategy, followed by a direct elemental halogenation with Br2/H2 O or I2/ethanol solution. The as-obtained PAN/Ag/AgX nanofiber mats exhibit exceptional photocatalytic activity toward degradation of organic pollutants. Furthermore, the flexibility enables it to be easily recovered after the reaction was completed. This work provides new insights into the fabrication of membrane-based photocatalysts on a large scale.

论文目录

文章来源

类型: 期刊论文

作者: Meng-Mo Ping,Shu-Jun Qiu,Gui-Juan Wei,Jun-Xue Liu,Zhao-Jie Wang,Shu-Tao Wang,Chang-Hua An

来源: Rare Metals 2019年05期

年度: 2019

分类: 工程科技Ⅰ辑

专业: 化学

单位: Tianjin Key Laboratory of Organic Solar Cells and Photochemical Conversion, School of Chemistry and Chemical Engineering, Tianjin University of Technology,School of Materials Science and Engineering, China University of Petroleum,Qingdao

基金: financially supported by the Key Project of Natural Science Foundation of Tianjin (No. 18JCZDJC97200)

分类号: O644.1;O643.32

页码: 361-368

总页数: 8

文件大小: 5410K

下载量: 6

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Monolith free-standing plasmonic PAN/Ag/AgX(X = Br, I)nanofiber mat as easily recoverable visible-light-driven photocatalyst
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